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The nucleus of this collection was created from papers given to the Association by Ann Pamela Cunningham around the time of her retirement as Regent. Several other Vice Regents followed her example and later donated their papers as well. These records were referred to as the "Early Records" since the time they were first established as an archival collection. A large portion of this collection is correspondence concerning the founding of the MVLA and the operation of Mount Vernon as a historic site. Other important resources are the appeals written by Ann Pamela Cunningham and the Vice Regents, governing documents, subscription or donation lists, printed material or publications, and bound volumes such as ledgers or scrapbooks. Individual items were added to the collection as they were acquired. The Early Records includes items dated 1852-1951, however the bulk of the material dates from 1858 to around 1880.

The bulk of this collection is correspondence to Mrs. Laughton concerning Mount Vernon and the work of the Mount Vernon Ladies' Association. Other material includes correspondence from Mrs. Laughton, formal reports and papers of the MVLA, personal correspondence and memoirs, photographs, printed material, and ephemera. The overall dates range from 1850 to 1891 with the bulk of the collection dating from the 1860s-1880s.

Collection of 80 photographs which belonged to Miss Sarah C. Tracy (later Mrs. Upton H. Herbert), resident secretary at Mount Vernon during the Civil War years. The pictures most of which are cartes de visite were collected by Miss Tracy; some were obviously presented to her, after the fashion of the day, and are inscribed. Besides the one of herself there are three of Mount Vernon which must date from the years of her residence. Others include Leeds Castle, the English seat of Thomas, Lord Fairfax; the President's House at the Soldiers' Home, Washington, D.C.; the Milwaukee residence of Mrs. Mitchell, Vice-Regent for Wisconsin; General Winfield Scott; General George B. McClellan; W. W. Corcoran of Washington, D.C.; George W. Riggs, Treasurer of the Association; Lord Fairfax; Prince Napoleon; Louis de Geofroy (of the French Legation, who accompanied Price Napoleon to Mount Vernon in August, 1861), inscribed; and Miss Nettie Chase, daughter of Hon. Salmon P. Chase of the Lincoln Cabinet. Also included are pictures of others, chiefly celebrated figures of the nineteenth century; these were probably acquired through gift or purchases, and not presented by the subjects themselves.