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Scope and Content: This collection was originally assembled by Esther Maria Lewis Chapin, who inherited some of the Washington and Custis papers but was also an avid collector. She reassembled family materials that were being dispersed nationwide, much of which was purchased at Anderson Galleries, sale 22001, 28-29 November 1927. The collection contains correspondence, legal documents, and financial records related primarily to the Custis and Lewis families. Much of the financial and legal materials focus on the construction of the New Tomb at Mount Vernon, as well as settling George Washington's estate.The dates of the material in this collection ranges from 1743-1852, with the bulk of the material dating between 1818-1829.

This collection contains college catalogs, commencement programs, form letters about registration, and other college publications; receipts for post office box and tuition; membership cards for Women Students' Cooperative Government Association and student activities; buttons with busts of George and Martha Washington honoring the bicentennial of Washington's birth; and other material from Nettles' college years.

This collection contains letters to and from Martha Washington that have been acquired by the MVLA since 1858. For more information, see content note for individual items. The collection grows organically as new items are acquired.

Collection of 80 photographs which belonged to Miss Sarah C. Tracy (later Mrs. Upton H. Herbert), resident secretary at Mount Vernon during the Civil War years. The pictures most of which are cartes de visite were collected by Miss Tracy; some were obviously presented to her, after the fashion of the day, and are inscribed. Besides the one of herself there are three of Mount Vernon which must date from the years of her residence. Others include Leeds Castle, the English seat of Thomas, Lord Fairfax; the President's House at the Soldiers' Home, Washington, D.C.; the Milwaukee residence of Mrs. Mitchell, Vice-Regent for Wisconsin; General Winfield Scott; General George B. McClellan; W. W. Corcoran of Washington, D.C.; George W. Riggs, Treasurer of the Association; Lord Fairfax; Prince Napoleon; Louis de Geofroy (of the French Legation, who accompanied Price Napoleon to Mount Vernon in August, 1861), inscribed; and Miss Nettie Chase, daughter of Hon. Salmon P. Chase of the Lincoln Cabinet. Also included are pictures of others, chiefly celebrated figures of the nineteenth century; these were probably acquired through gift or purchases, and not presented by the subjects themselves.

Letter dated 7 January 1773, from George Washington of Mt. Vernon to Rev. Jonathan Boucher (tutor to John Parke Custis, Washington's step-son) regarding Washington's suggestions for where Custis should attend college. It includes the following comments about William and Mary: