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The bulk of the Charles A. Derby papers consists of Derby family correspondence. Approximately twenty-eight letters were written by Charles A. Derby (dated 1844-1862) and cover the period from late boyhood up to his death in battle in 1862. Included are letters (dated 1846-1847) written while he was a cadet at VMI, as well as correspondence dating from his careers as a teacher and Episcopal clergyman. Two items were written during his brief service in the Confederate Army.

This collection includes correspondence while Jamison was Secretary of War of South Carolina, 1861; scattered letters and papers pertaining to the South Carolina Secession Convention of which he was president, and papers related to his tenure as presiding judge of the military court of Gen. Beauregard's Corps, 1862-1864. Robert Woodward Barnwell and Lawrence Massillon Keitt are among the correspondents.

The nucleus of this collection was created from papers given to the Association by Ann Pamela Cunningham around the time of her retirement as Regent. Several other Vice Regents followed her example and later donated their papers as well. These records were referred to as the "Early Records" since the time they were first established as an archival collection. A large portion of this collection is correspondence concerning the founding of the MVLA and the operation of Mount Vernon as a historic site. Other important resources are the appeals written by Ann Pamela Cunningham and the Vice Regents, governing documents, subscription or donation lists, printed material or publications, and bound volumes such as ledgers or scrapbooks. Individual items were added to the collection as they were acquired. The Early Records includes items dated 1852-1951, however the bulk of the material dates from 1858 to around 1880.

Includes Ledgers, vouchers, accounts, correspondence, and other financial records dating from the opening days of the Institute through the early 20th century. These records are a good source of information for tracing early purchases of goods and services; local Lexington and Rockbridge County businesses/artisans/craftsmen appear in vouchers.