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The A. Jane Duncombe Architectural Papers span the years 1952 to 2002. The papers consist primarily of architectural drawings, as well as some printed material including plan sheets, articles, and printouts of digital images. The collection documents various residential and other projects upon which Duncombe worked, one in Illinois and the rest in California.

The Beverly Willis Architectural Collection span the years 1954 to 1999 and are comprised primarily of records documenting Willis' work as an architect in San Francisco between 1960 and 1990. The collection documents the application of computers to architectural design and land analysis, the development of CARLA (Computerized Approach to Residential Land Analysis) in the 1970s, the history of twentieth-century urban planning, particularly in San Francisco; and the contribution of women to twentieth-century American architecture. Willis, a noted artist, photographer, teacher, and writer, employed the full range of visual arts and design skills to influence and guide architectural projects of major significance.

The Historical Photograph Collection is largely comprised of materials created by or for the Mount Vernon Ladies' Association. Photographers primarily include staff members and contract photographers. The collection spans the 1930s to the 2000s and includes analog material made up of a variety of sizes of film negatives providing a visual history of the Mansion, outbuildings, tombs, grounds, events, visitors, collection objects, personnel, restoration, and changes throughout the estate.

This collection contains letters to and from George Washington that have been aquired by the MVLA since 1858. For more information, see content note for individal items. The collection grows organically as new items are acquired.