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The papers of Anna Maria (Campbell Hickman) Otis Mead Chalmers (1809-1891) and her family offer a deep look into a 19th century American family with a sharp focus on enslaved and formerly enslaved persons. The collection documents the life of a young, widowed woman, Anna Maria Mead Chalmers, who was the granddaughter of General William Hull (1753-1825). She was a mother of four children and became a businesswoman in Richmond, Virginia. She was a writer, an editor of the Southern Churchmen, an educator and founder of Mrs. Mead's School for Young Ladies, and a director of The Southern Churchmen Cot ("Retreat for the Sick"), a hospital for children. Anna Maria's family enslaved people who are represented in the papers including Othello "Tillo" Freeman (1790's-1860's?). It includes a letter from William written in [1875], who was their carriage driver, and letters about Sam the fiddler, who settled on the farm after escaping harsher enslavement in Louisianna, and Jordan who was described as being hired out in a letter dated September 8, 1841 from Thomas R. Blair.

This collection includes correspondence between John Augustine Washington III and his mother and wife, as well as other family members, mostly dealing with family matters and running Mount Vernon.

The Bushrod Washington Family Papers consist of documents gathered by the descendants of the first President of the United States, George Washington. The collection comprises an assortment of correspondence and legal documents documenting the lives and property ownership of several branches of the Washington family. The collection is organized into five series: Correspondence, Legal Documents, Social, Miscellaneous, and Indenture Notices (Land Deeds).

This collection consists of papers inherited and collected by Washington family descendants. Many were purchased in 1927 at auction to reunite Washington family correspondence. The collection includes correspondence, financial documents and legal documents that relate primarily to the Custis and Lewis families, but include other items related to Virginia history. Charles and Peter Chapin, the previous owners of this collection, descended from Eleanor Parke Custis and Lawrence Lewis through Esther Maria Lewis and Charles Chapin. This collection was originally assembled by Esther Maria Lewis Chapin who inherited some of the Washington/Custis papers, but was also an avid collector and brought back together family items that were being dispersed nationwide. This collection is an example of that effort; much of which was at auction in 1927 (Anderson Galleries, sale 2201, 28-29 November 1927).