- "George Washington" Miniseries Collection, 1981/19861
- Anniversaries and Commemorations Collection, 1981/200055
- Audio Visual Collection, 1928/2015345
- Beebe collection of Washington family papers, 1818/1861, bulk 1840/185043
- Bushrod Washington family papers, 1662/1835267
- Chapin collection of Washington & Custis family documents, 1758/182922
- Early Records of the Mount Vernon Ladies' Association, 1853/1951, bulk 1853/18755,388
- Edith Sprouse Subject Files, 1960/198622
- Elizabeth Bordley Gibson collection, 1794/1851219
- Emma Read Ball Genealogical Research Files, 1911/191235
- Esther Maria Lewis Chapin collection of Washington family documents, 1743/185293
- Financial Records of the Mount Vernon Ladies' Association, 1858/2015560
- Frances Abbott Lyon Papers, 1976/19835
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/2017430
- George Washington Memorial Parkway History Collection, 1900/20018