- Alexander Family Papers
1800-18901
- Bradford Laidley Papers, 1755/19911
- C. L. Worthington Papers, 1752/19381
- Cassie Moncure Lyne Scrapbook, 1930/19431
- Cynthia Beverley Tucker Washington Coleman Papers, 1834/19281
- Ellen Washington Bellamy Collection, 1860/19041
- Frances Packette Todd Papers, 1800/19851
- Henrietta S. Fitzhugh Collection, 1827/2003, bulk 1827/20031
- James B. Lynch Collection (MS022), 1974/19931
- Mary E. Heironimus, Collector, Records regarding George Washington and Other Material, 1799/20141
- Roane Family Papers, 1880/1973, bulk 19501
- Roy Bird Cook (1886-1961), Collector, Papers regarding General Joseph A.J. Lightburn and Other Material, 1774/1960, bulk 1939/19601
- Washington Family Devotional Book and Genealogical Notes, 1940/19501
- William A. Alexander Papers, 1833/1900, bulk 1842/18851