- 8th Evacuation Hospital collection, 1941/20114
- A. E. Dick Howard papers on the Virginia Commission on Constitutional Revision, 1968/1971299
- A. E. Dick Howard papers, 1928/20171,390
- A. J. Gustin Priest papers, 1919/197615
- Addison H. Smith papers, 1917/1970, bulk 1917/192222
- Additional Papers of S. Vernon McCasland
1928-195413
- African American Hugh Carr family, River View Farm, and the Papers of the Ivy Creek Foundation, 1916/198815
- African American man tintype portrait, 1865/19001
- Albert Frederick Wilson papers, 1840/193417
- Albert R. Gallatin papers, 1795/18282
- Alderman family papers, 1779/196115
- Alexander G. Gilliam collection of University of Virginia history papers, 1921/201983
- Alexander Gilliam diaries, 19435
- Alfonso García Robles papers, 1978/198820
- Alfred Tennyson papers, 1875/18762