- Ancient Coins, 1956/19933
- Dr. Charles Ferguson McRae Collection, 1935/19931
- Dr. Herbert J. Sipe, Jr. Papers, 1927/201927
- Dr. Ralph A. Rossum Papers, 1988/19927
- Dr. Walter Taylor Reveley II Papers, 1963/19931
- Elizabeth Carrington Eggleston Papers, 1899/19942
- Hampden-Sydney Library Records, 1930/20123
- Josiah Bunting III Papers, 1972/19984
- Log Cabin School Collection, 1966/20224
- Paul L. Grier Vertical Files, 1775/19881
- Records of the Merrill's Marauders Proud Descendants Association, 1944/20209
- Records of the Philanthropic, Union, and Union-Philanthropic Literary Societies, 1789/20071
- Rev. S.M. Engle Papers, 1865/19371
- Richard McClintock Collection, 1960/20151
- Royal E. Cabell Jr. Papers, 1992/19992