- Albert J. Wasserman Papers, 1925/20031
- Albert S. Armentrout Collection, 1965/20091
- Alexander "Sandy" Gilliam papers, 1985/20161
- Alexander G. Gilliam collection of University of Virginia history papers, 1921/20191
- Alexandria Antique Arts Association Collection (MS134), 1971/19991
- Alexandria Black Family Reunion Digital Collection, 1937/20051
- Alexandria Gazette I (MS331), 1942/19961
- Alexandria History Collection (MS240), 1767/20081
- Alexandria Library Board Records (MS416), 1937/20201
- Alexandria Library Company Records (MS002), 1794/20071
- Alexandria Library Records (MS098), 1937/20131
- Alexandria Recital Series Papers (MS312), 1980/20021
- Alfred A. Bolton, Papers regarding History of Management and Other Material, 1900/20071
- Alfred C. Payne Collection, 1917/20031
- Alice Cartledge Cornett, Journalist, Papers, 1945/2017, bulk 1973/19921