- "George Washington" Miniseries Collection, 1981/19861
- Anniversaries and Commemorations Collection, 1981/20002
- Audio Visual Collection, 1928/20158
- Edith Sprouse Subject Files, 1960/19864
- Financial Records of the Mount Vernon Ladies' Association, 1858/201523
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/201711
- George Washington Memorial Parkway History Collection, 1900/20013
- Guest Books and Visitor Registers, 1850/20162
- Historic ephemera collection, 1796/19863
- Historic manuscript collection, 1601/19331
- Historical Photograph Collection, 1850/20106
- John Augustine Washington III and family papers, 1789/19942
- Kellogg Foundation Files, Farm Project, 1984/19992
- Land Records of the MVLA, 1858/20061
- Licensing Department Files, 1984/20144