- Administrative Management Society records, 1941/1987, bulk 1941/19871
- Admiral Thomas J. Lopez Papers, 1973/20146
- Admissions Office student recruitment materials, 1950/20191
- Adolphus DeBussey, Soldier, Civil War Letters, 1861/1998, bulk 1861/18711
- Aerial Photographs of the Virginia Dept. of Transportation,, 1930/20151
- African American Hugh Carr family, River View Farm, and the Papers of the Ivy Creek Foundation, 1916/19881
- African American programs and photographs from Roanoke, and Wytheville, Virginia, 1954/19771
- Agnes M. Marshall/American Association of Neuroscience Nurses Papers, 1967/20091
- Agnes Wolf papers, 1966/20067
- Agra Bennett, Papers Regarding Estate and Residence, 1967/20101
- Agricultural Extension Service Records, 1914/19801
- Al Gross Papers, 1909/200012
- Alan Bowne papers, 1964/1991, bulk 1980/19894
- Alan Clarke Railroad Research Papers, 1861/20126
- Alastair Reid Poem, 1973/19742