- Adam Empie Papers, 1811/2004, bulk 1811/18503
- Addison H. Smith papers, 1917/1970, bulk 1917/19222
- Additional Louis J. Halle, Jr. Papers
1938-198719
- Adele Blow Chatfield-Taylor family papers, 1899/197722
- Adele Goodman Clark papers, 1849/197853
- Administration records collection, 1776/19762
- Administrative Management Society records, 1941/1987, bulk 1941/19874
- Admissions Office student recruitment materials, 1950/20191
- Adolphus DeBussey, Soldier, Civil War Letters, 1861/1998, bulk 1861/18711
- Aerial Photographs of the Virginia Dept. of Transportation,, 1930/20151
- African American GI's Vietnam and West Germany Scrapbook, 1960/19691
- African American Hugh Carr family, River View Farm, and the Papers of the Ivy Creek Foundation, 1916/19881
- African American programs and photographs from Roanoke, and Wytheville, Virginia, 1954/19771
- Agnes Smith (1906-1994), Author, Correspondence, Manuscripts, and Publications, 1920/19701
- Agnes Smith (1906-1994), Author, Literary Manuscripts, 1930/19701