- Papers of the Superintendent and Resident Director, 1850/1996182
- Restoration Files for the Historic Structures Report, 1750/2005161
- Papers of the Mount Vernon Ladies' Association, 1858/2016151
- Mount Vernon Black and White Film Collection, 1933/200551
- Operation Overview Collection, 1953/198340
- Financial Records of the Mount Vernon Ladies' Association, 1858/201535
- Papers of Christine Meadows, Curator, 1960/199730
- Historical Photograph Collection, 1850/201025
- Publications Committee Collection, 1951/199715
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/201714
- Publications and Printed Material of the Mount Vernon Ladies' Association, 1854/201611
- Audio Visual Collection, 1928/20159
- Historic ephemera collection, 1796/19868
- John Augustine Washington III and family papers, 1789/19948
- Publications - History of Mount Vernon and George Washington, 1854/20128