- Blair-Weindel-Schrader Family Papers, 1943/19981
- Buckhorn Coal Company Records, 1880/19611
- Carroll and Wythe Counties Industries Collection, 1937/19801
- Episcopal Diocese of Southwestern Virginia Records II, 1913/19671
- Episcopal Diocese of Southwestern Virginia Records, 1866/2004, bulk 1919/19691
- Historical Maps Collection, 1500/20231
- John Henry Johnson Scrapbook, 1918/19581
- Madison E. Marye Papers, 1932/20071
- Richard B. Dickenson Papers,, 1931/2004, bulk 1964/20001
- Roanoke Appalachian Trail Club Records, 20251
- Smithey & Boynton, Architects & Engineers Records, 1922/19851
- William C. Wampler Congressional Papers, 1953/1990, bulk 1967/19821