- Allison Kenneth Scribner Papers, 1946/19762
- Alpha Sigma Alpha Collection, 1933/20185
- Althea Hunt Papers, 1926/196119
- Alton D. Brashear papers, 1935/19551
- Alumni Association Photograph Collection, 1960/2010, bulk 1970/19901
- Alumni Association Records, 1833/2014, bulk 1950/200550
- Alumni Association Records, 1924/201611
- Alumni Association Records, 1950/20074
- Alumni and VMI certificates and citations collection, 1860/20133
- Alumni biographical files - University of Virginia School of Law, 1901/19971
- Alvena V. Seckar, Author and Artist, Artwork and Papers, 1940/19681
- Alvena V. Seckar, Author and Artist, Manuscripts and Correspondence, 1940/19681
- Alvena V. Seckar, Author and Artist, Writings, Photographs, Scrapbooks, and Other Material, 1927/200513
- Alvin D. Chandler Naval Record, 1925/19511
- Alvin Duke Chandler Papers, 1896/1984, bulk 1950/19603