- Alexandria History Collection (MS240), 1767/200829
- Alexandria Hospital School of Nursing records, 1894/19871
- Alexandria Library Company Records (MS002), 1794/20075
- Alexandria National Bank Collection (MS193), 1904/19781
- Alexandria Office of Sheriff Jail Records (MS054), 1891/19481
- Alexandria, Virginia City Records (MS019), 1750/1983, bulk 1825/18751
- Alfred A. Bolton, Papers regarding History of Management and Other Material, 1900/200733
- Alfred C. Garnett, Jr. Papers
1868-194510
- Alfred C. Payne Collection, 1917/200312
- Alfred Dickinson Barksdale Papers
1893-19406
- Alfred Dickinson Barksdale Papers
1905-19736
- Alfred P. Upshur collection, 1909/19531
- Alfred R. Armstrong Papers, 1928/19761
- Alfred W. Lawson Collection, 1913/19481
- Alice Constance Burford Booth Papers, 1940/19684