- Adele Blow Chatfield-Taylor family papers, 1899/19772
- Adele Goodman Clark papers, 1849/19783
- Alexander Farish Robertson Papers, 1867/19316
- Alexander Haight family collection, 1764/19761
- Alleghany Chapter, National Society of the Daughters of the American Revolution Records, 1890/20221
- Alumni Association Records, 1833/2014, bulk 1950/20052
- American Association of University Women, Norfolk Branch (AAUW) Records, 1902/20001
- Ancella Bickley, Historian, Research Papers regarding African-Americans, 1775/2018, bulk 1970/201113
- Anne Atkinson Chamberlayne Collection., 1742/19631
- Armistead Boothe Papers (MS164), 1803/19902
- Arthur E. Scott photograph collection1
- Arthur E. Scott photograph collection, 1910/19761
- Austin-Twyman Papers, 1765/193913
- Bailey-Law Collection, 1825/19718
- Bell, Kent, Cloyd, Withrow Family Collection, 1780/19981