- Albert Frederick Wilson papers, 1840/19341
- Alderman family papers, 1779/19611
- Alexander Wylie Moore miscellaneous papers, 1896/19501
- Alexandria Hospital School of Nursing records, 1894/19871
- Alfred Oscar Elzner sketch book and album, 1883/19231
- Alumni Day records, 1900/19791
- Alumni biographical files - University of Virginia School of Law, 1901/19971
- American Lung Association of Virginia (ALAV) collection, 1907/20041
- Arlene Keeling Collection, 1861/20061
- Armistead Mason Dobie papers, 1902/19651
- Armstead L. Robinson papers, 1848/2001, bulk 1967/19921
- Arthur J. Morris memorabilia, 1884/19921
- Aubrey E. Strode papers, 1861/19691
- Avent family papers, 1905/19821
- Barbara Brodie Nursing History Collection Additions, 1890/19891