- Alumni Association Records, 1833/2014, bulk 1950/20051
- Austin-Twyman Papers, 1765/193931
- Blow Family Papers, 1613/1960, bulk 1770/18756
- Borland Family Papers, 1771/19401
- Brown, Coalter, Tucker Papers (I), 1790/19293
- Brown, Coalter, Tucker Papers (II), 1791/19208
- Coleman-Kimbrough papers, 1870/19921
- Cook-Luttrell Papers, 1848/18904
- Edward "Teddy" Bolton Tucker Papers, 1760/2007, bulk 1800/19002
- Gloucester Circuit of the Methodist Church Records, 1825/19103
- Grigsby-Galt Papers, 1736/1982, bulk 1840/19302
- Hamilton Family Papers, 1892/2003, bulk 1930/20031
- Hart collection, 1762/19391
- Henkel Family Papers, 1783/18741
- Henry Denison Cole Papers, 1786/19395