- Virginia Counties Collection, 1600/2000, bulk 1730/189040
- Historic newspapers collection, 1757/19577
- Morley Jeffers Williams Collection, 1602/19677
- Alexandria History Collection (MS240), 1767/20086
- Richard Billups Papers, 1705/1857, bulk 1774/18225
- Peter family papers, 1722/19324
- Wilkin Family Papers, 1757/1922, bulk 1780/18704
- Barry S. Martin collection of historical manuscripts and documents, 1771/18303
- Brooke County (W. Va.) Court Records and Miscellaneous Papers, 1780/19183
- Bushrod Washington family papers, 1662/18353
- Charles Campbell Papers, 1743/18963
- Galt Papers (I), 1745/18923
- Galt Papers (III), 1750/19913
- Jerdone Family papers, 1753/18903
- Jim Comstock, Newspaper Editor and Collector, Papers, 1650/2003, bulk 1850/19953