- Jack Sandy Anderson, Compiler, Local History Articles and Genealogy Papers, 1600/2011, bulk 2000/20081
- James Edwin Green, Photographer, Glass Plate Negatives and Other Material, 1900/1925, bulk 1900/19181
- James M. Guiher, Jr., Papers, 1835/2014, bulk 1927/19761
- Jan Karon papers, 1918/2018, bulk 1964/20181
- John D. Hoblitzell, Jr. (1912-1962), Politician, Papers, 1956/19621
- Naval Account Book, 1660/17111
- Ollen Lawrence Burnette, Jr. papers, 1815/20141
- Richard A. Rutyna Papers, 1763/20111
- Richard J. DeMartino papers, 1910/19651
- Richard Lee Morton papers, 1756/2006, bulk 1930/19691
- Robb-Bernard Papers, 1665/1980, bulk 1850/19501
- Saint Andrew's Society of Washington, D.C. records, 1861/19951
- Samuel H. Yonge papers, 1890/19351
- Sheet Music Collection, 1827/19742
- Thomas G. and Louise Rowe Pullen Collection, 1655/17912