- Appomattox Manor Music Collection, 1800/1940, bulk 1850/19101
- Bound Music Collection, 1800/19701
- Edward Vitale violin music collection, 1886/19511
- Frances Breeze Music Collection, 1890/19801
- John Alexander Graham Papers, 1910/1947, bulk 1915/19473
- Josephine W. Shinholser Collection of Sheet Music, 1890/19971
- Katie L. Hopkins Collection of Sheet Music and Songbooks, 1890/19101
- Music: Songs, 1896/19871
- Racial and Ethnic Ephemera Collection, 1778/20051
- Richard Wright collection, 1806/20171
- Ruth and Lowell Toliver Collection of Newman Family Papers, 1875/20051
- Sheet Music Collection, 1827/19741
- Stonewall Jackson papers, 1844/19151
- VMI sheet music collection, 1857/19301