- Board of Visitors records, 1757/20231
- Campbell Family Papers, 1726/19201
- Collection of French Language Manuscripts, 1633/1942, bulk 1633/19421
- James Madison, Sr. Papers, 1792/19311
- John Garland Pollard Papers, 1683/1968, bulk 1856/19371
- Myers-Burrage-Graham papers (I), Group A, 1776/19251
- Phi Beta Kappa, Alpha Chapter Records, 1776/2013, bulk 1888/19551
- Richard Lee Morton papers, 1756/2006, bulk 1930/19691
- United States Federal Nineteenth Century Government Publications, 1826/18781
- William Booth Taliaferro Papers, 1811/19541
- William F. Willoughby Papers, 1818/1955, bulk 1891/19371