- Frances Breeze Music Collection, 1890/19801
- Grace Warren Landrum Papers, 1890/19951
- Guy Family Papers, 1900/19881
- Heinz and Gertrud Siegel Elber papers, 1918/20181
- Helen L. Johnson Papers, 1925/1982, bulk 1925/19401
- Henry Denison Cole Papers, 1786/19391
- J. Wilfred Lambert Papers, 1920/19741
- Janet C. Kimbrough Williamsburg Area History Collection, 1873/19941
- John Alexander Graham Papers, 1910/1947, bulk 1915/19471
- John Branch Green Papers, 1924/19291
- John Tyler Papers, 1840/19311
- Julia W. Oxrieder Papers, 1877/19981
- Lloyd H. and Ruth Elizabeth Williams Papers, 1917/2008, bulk 1947/19591
- Matthew Whaley School Collection, 1850/2012, bulk 1880/19601
- May Day Records, 1926-1999, 1927/1999, bulk 1930/19391