- A. G. Stuart Notebook, 18721
- A.S. Hammack papers, 1864/19541
- Abbot E. Smith Papers, 1930/19391
- Agnes Davis Shipley papers, 19361
- Alexander W. Archer Textbook, 18251
- Alfred R. Armstrong Papers, 1928/19761
- Anonymous dating diary, 1943/19471
- Anthony Esler Papers, 1962/19801
- Archibald F. Ward, Jr. Papers, 1939/2007, bulk 1945/19601
- Archibald Stewart Notebook, 17051
- Arithmetic Notebook, 18321
- Arithmetic Notebook, I, 1780/18201
- Arithmetic Notebook, II, 18331
- Armistead C. Gordon Notes about the Bench and Bar of Virginia, 19091
- Asa Dupuy Notebook, 1819/18211