- Armistead-Cocke Papers, 1680/19171
- Baird Family Papers, 1656/1922, bulk 1656/18481
- Civil War Collection, 1856/19381
- Gloucester Circuit of the Methodist Church Records, 1825/19101
- Harriet P. Shelden Recipe Book, 1820/19001
- John Tayloe Perrin Papers, 1770/19311
- Jones Family Papers, 1826/19161
- Molly Elliot Seawell Papers, 1859/2001, bulk 1889/19161
- Nicolson Family Ledgers and Journals, 1802/19141
- Roane Family Papers, 1880/1973, bulk 19501
- Taliaferro Family Papers, 1846/18951
- The Reverend Henry Gardiner Lane Memorial Collection, 1799/19381
- Warner T. Jones Papers, 1818/18911
- William Booth Taliaferro Papers, 1811/19541
- William K. Perrin Papers, 1732/1902, bulk 1820/18581