- Adam Empie Papers, 1811/2004, bulk 1811/18501
- Alumni Association Records, 1833/2014, bulk 1950/20051
- Benjamin Stoddert Ewell Papers, 1784/1934, bulk 1830/18921
- Blow Family Papers, 1613/1960, bulk 1770/18751
- Board of Visitors records, 1757/20231
- Borland Family Papers, 1771/19401
- College Papers Collection, 1880/19991
- Commencement Exercises collection, 1831/20241
- Cynthia Beverley Tucker Washington Coleman Papers, 1834/19281
- Edwin Taliaferro Collection, 1860/19711
- Faculty Assembly Records, 1729/20081
- Grigsby-Galt Papers, 1736/1982, bulk 1840/19301
- Hall Family Papers, 1810/20071
- Henry Denison Cole Papers, 1786/19391
- John Lesslie Hall Papers, 1885/19281