- Alumni and VMI certificates and citations collection, 1860/201337
- Geo. Gregory Smart collection of Washington and Mount Vernon ephemera, 1793/20178
- Office of Communications and Marketing subject files, 19504
- VMI diplomas collection, 1842/19784
- Historic ephemera collection, 1796/19862
- Jesse H. Heath, Jr. collection, 1941/19932
- John T. L. Preston papers, 1806/18892
- Soldiers' memorabilia and military service related manuscripts, 1917/19942
- Albert D. Davis papers, 1930/19521
- Alfred P. Upshur collection, 1909/19531
- Allan T. Gwathmey collection, 1914/19491
- Amos Koontz Papers I, 1809/1965, bulk 1936/19651
- Anatole and Vladimir Kalichevsky Papers, 1871/19551
- Augustine Smith Papers, 1787/17931
- Betty Coe Cinquegrana papers, 1960/20141