- Alumni and VMI certificates and citations collection, 1860/20132
- Betty Coe Cinquegrana papers, 1960/20141
- Blackley Family papers, 1830/20201
- Carter Lowance Papers, 1860/1993, bulk 1942/19881
- Caskie Stinnett Papers, 1919/1998, bulk 1950/19931
- Charles Edward Gary, Jr. Papers, 1870/2000, bulk 1940/19801
- Christopher Bram Papers, 1968/2014, bulk 1975/20001
- Davis, Kline, and Hutton Family papers, 1816/19771
- Dorothy McKinley Spooner Garber Papers, 1925/19781
- Duff Green, Jr. collection, 1929/19791
- Edward Belvin Collection of Williamsburg and James City County materials, 1874/19871
- Elmon T. Gray collection, 1931/20101
- F.H.C. Society Collection, 1911/20121
- Glenna G. Shiflett Papers, 1961/19931
- Grigsby-Galt Papers, 1736/1982, bulk 1840/19301